English

Antiferromagnetic ground state in the MnGa$_4$ intermetallic compound

Materials Science 2018-05-09 v2

Abstract

Magnetism of the binary intermetallic compound MnGa4_4 is re-investigated. Band-structure calculations predict antiferromagnetic behavior in contrast to Pauli paramagnetism reported previously. Magnetic susceptibility measurements on single crystals indeed reveal an antiferromagnetic transition at TN=393T_N=393 K. Neutron powder diffraction and 69,71^{69,71}Ga nuclear quadrupole resonance spectroscopy show collinear antiferromagnetic order with magnetic moments alligned along the [111] direction of the cubic unit cell. The magnetic moment of 0.80(3)μB\mu_B at 1.5 K extracted from the neutron data is in good agreement with the band-structure results.

Keywords

Cite

@article{arxiv.1802.03256,
  title  = {Antiferromagnetic ground state in the MnGa$_4$ intermetallic compound},
  author = {V. Yu. Verchenko and A. A. Tsirlin and D. Kasinathan and S. V. Zhurenko and A. A. Gippius and A. V. Shevelkov},
  journal= {arXiv preprint arXiv:1802.03256},
  year   = {2018}
}
R2 v1 2026-06-23T00:17:02.309Z