Multilayer graphene with different stacking sequences has emerged as a powerful setting for correlated and topological phases. In parallel, progress in graphene heterostructures with magnetic or correlated materials-most notably the Kitaev candidate α-RuCl3-has demonstrated charge transfer, magnetic proximity effects, and interfacial reconstruction, creating new opportunities for engineered quantum systems. Motivated by these developments, we explore a three-dimensional analogue in which α-RuCl3 layers are inserted directly into the van der Waals gaps of graphite, forming an intercalated system. Here, we report the successful synthesis and comprehensive characterization of graphite intercalated with α-RuCl3. Using a combination of X-ray diffraction, quantum oscillation measurements, and first-principles electronic structure calculations, we study the structural and electronic properties of these intercalated crystals. Our results demonstrate that graphite intercalated with α-RuCl3 offers a robust route to develop three-dimensional materials with access to novel correlated and topological states.
@article{arxiv.2512.03147,
title = {$\alpha$-RuCl$_3$ intercalated into graphite: a new three-dimensional platform for exotic quantum phases},
author = {Aleksandar Razpopov and Shirin Mozaffari and Takahiro Matsuoka and Matthew Cothrine and Nan Huang and Roser Valentí and David Mandrus},
journal= {arXiv preprint arXiv:2512.03147},
year = {2026}
}
Comments
14 pages, 10 figures, including supplementary information