English

$\alpha$-RuCl$_3$ intercalated into graphite: a new three-dimensional platform for exotic quantum phases

Strongly Correlated Electrons 2026-02-03 v2

Abstract

Multilayer graphene with different stacking sequences has emerged as a powerful setting for correlated and topological phases. In parallel, progress in graphene heterostructures with magnetic or correlated materials-most notably the Kitaev candidate α\alpha-RuCl3_3-has demonstrated charge transfer, magnetic proximity effects, and interfacial reconstruction, creating new opportunities for engineered quantum systems. Motivated by these developments, we explore a three-dimensional analogue in which α\alpha-RuCl3_3 layers are inserted directly into the van der Waals gaps of graphite, forming an intercalated system. Here, we report the successful synthesis and comprehensive characterization of graphite intercalated with α\alpha-RuCl3_3. Using a combination of X-ray diffraction, quantum oscillation measurements, and first-principles electronic structure calculations, we study the structural and electronic properties of these intercalated crystals. Our results demonstrate that graphite intercalated with α\alpha-RuCl3_3 offers a robust route to develop three-dimensional materials with access to novel correlated and topological states.

Keywords

Cite

@article{arxiv.2512.03147,
  title  = {$\alpha$-RuCl$_3$ intercalated into graphite: a new three-dimensional platform for exotic quantum phases},
  author = {Aleksandar Razpopov and Shirin Mozaffari and Takahiro Matsuoka and Matthew Cothrine and Nan Huang and Roser Valentí and David Mandrus},
  journal= {arXiv preprint arXiv:2512.03147},
  year   = {2026}
}

Comments

14 pages, 10 figures, including supplementary information

R2 v1 2026-07-01T08:06:25.072Z