English

Accurate interaction energies from perturbation theory based on Kohn-Sham model

Chemical Physics 2007-05-23 v1 Atomic and Molecular Clusters

Abstract

The density-functional based symmetry-adapted perturbation theory [SAPT(DFT)] has been applied to the argon, krypton, and benzene dimers. It is shown that--at a small fraction of computational costs--SAPT(DFT) can provide similar accuracies for the interaction energies as high-level wave-function based methods with extrapolations to the complete basis set limits. This accuracy is significantly higher than that of any other DFT or DFT-based approaches proposed to date.

Keywords

Cite

@article{arxiv.physics/0501023,
  title  = {Accurate interaction energies from perturbation theory based on Kohn-Sham model},
  author = {Rafał Podeszwa and Krzysztof Szalewicz},
  journal= {arXiv preprint arXiv:physics/0501023},
  year   = {2007}
}

Comments

4 pages, 3 figures

R2 v1 2026-07-22T19:02:27.238Z