English

Accelerating inverse materials design using generative diffusion models with reinforcement learning

Chemical Physics 2025-11-06 v1

Abstract

Diffusion models promise to accelerate material design by directly generating novel structures with desired properties, but existing approaches typically require expensive and substantial labeled data (>>10,000) and lack adaptability. Here we present MatInvent, a general and efficient reinforcement learning workflow that optimizes diffusion models for goal-directed crystal generation. For single-objective designs, MatInvent rapidly converges to target values within 60 iterations (\sim 1,000 property evaluations) across electronic, magnetic, mechanical, thermal, and physicochemical properties. Furthermore, MatInvent achieves robust optimization in design tasks with multiple conflicting properties, successfully proposing low-supply-chain-risk magnets and high-κ\kappa dielectrics. Compared to state-of-the-art methods, MatInvent exhibits superior generation performance under specified property constraints while dramatically reducing the demand for property computation by up to 378-fold. Compatible with diverse diffusion model architectures and property constraints, MatInvent could offer broad applicability in materials discovery.

Keywords

Cite

@article{arxiv.2511.03112,
  title  = {Accelerating inverse materials design using generative diffusion models with reinforcement learning},
  author = {Junwu Chen and Jeff Guo and Edvin Fako and Philippe Schwaller},
  journal= {arXiv preprint arXiv:2511.03112},
  year   = {2025}
}
R2 v1 2026-07-01T07:22:14.932Z