A minimal model for kinetic arrest
Statistical Mechanics
2009-11-13 v1 Soft Condensed Matter
Abstract
To elucidate slow dynamics in glassy materials, we introduce the {\it Figure-8 model} in which hard blocks undergo Brownian motion around a circuit in the shape of a figure-8. This system undergoes kinetic arrest at a critical packing fraction , and for long-time diffusion is controlled by rare, cooperative `junction-crossing' particle rearrangements. We find that the average time between junction crossings , and hence the structural relaxation time, does not simply scale with the configurational volume of transition states, because also depends on the time to complete a junction crossing. The importance of these results in understanding cage-breaking dynamics in glassy systems is discussed.
Cite
@article{arxiv.0804.2060,
title = {A minimal model for kinetic arrest},
author = {Prasanta Pal and Corey S. O'Hern and Jerzy Blawzdziewicz and Robin Stinchcombe},
journal= {arXiv preprint arXiv:0804.2060},
year = {2009}
}
Comments
4 pages, 4 figures