English

A fluctuation-free pathway for a topological magnetic phase transition

Materials Science 2025-12-30 v1

Abstract

Topological magnetic textures are particle-like spin configurations stabilized by competing interactions. Their formation is commonly attributed to fluctuation-driven, first-order nucleation processes requiring activation over a topological energy barrier. Here, we demonstrate an alternative barrier- and fluctuation-free pathway for nucleating topological magnetic textures, triggered in our experiments by an excitation-induced spin reorientation transition. By combining x-ray imaging, scattering and micromagnetic simulations, we show that the system follows a deterministic cascade of symmetry-breaking phase transitions after excitation. First, the system undergoes a second-order phase transition from a homogeneous state to weak stripe domains, then a first-order transition to topologically trivial bubbles, and finally a topological switching event into skyrmionic textures. Through simulations, we generalize our findings and demonstrate that this pathway is active in a vast range of low-anisotropy materials. This previously unrecognized, spontaneous transition pathway suggests strategies for rapid, low-energy generation of topological spin textures and points to a general role of intrinsic modulational instabilities in phase transitions beyond magnetism.

Keywords

Cite

@article{arxiv.2512.22947,
  title  = {A fluctuation-free pathway for a topological magnetic phase transition},
  author = {Riccardo Battistelli and Lukas Körber and Kai Litzius and Matthieu Grelier and Krishnanjana Puzhekadavil Joy and Michael Schneider and Steffen Wittrock and Daniel Metternich and Tamer Karaman and Lisa-Marie Kern and Christopher Klose and Simone Finizio and Josefin Fuchs and Christian M. Günther and Tim A. Butcher and Karel Prokeš and Raluca Boltje and Manas Patra and Sebastian Wintz and Markus Weigand and Sascha Petz and Horia Popescu and Jörg Raabe and Nicolas Jaouen and Stefan Eisebitt and Vincent Cros and Bastian Pfau and Johan H. Mentink and Nicolas Reyren and Felix Büttner},
  journal= {arXiv preprint arXiv:2512.22947},
  year   = {2025}
}

Comments

44 pages, 19 figures (of which 5 figures are in main text, 4 in Supplementary Information and 10 are Extended Data Figures). The raw data, source data and analysis code for all figures are available at https://zenodo.org/doi/10.5281/zenodo.18004538